所属学院：

材料与能源学院

导师类别：

博士生导师/硕士生导师

科研方向：

纳米催化、能源材料

联系方式：

yongxu@gdut.edu.cn

招生学院：

材料与能源学院

个人简述

课题组聚焦于贵金属纳米催化剂的设计、可控合成、结构调控及构效关系研究。利用多种原位表征方法研究催化剂界面构效关系及催化作用机理，并积极探索在石油化工、新型清洁能源及环境保护等领域的应用。主要研究方向：

1、贵金属纳米催化剂可控合成与结构调控；

2、无机功能纳米催化剂的表界面改性及其在能源与催化方面的应用

学科领域

科学学位：材料科学与工程

专业学位：材料工程

教育背景

2013年6月 中国科学技术大学可再生洁净能源专业 获博士学位

2011年9月-2012年9月 意大利国家核物理研究院Frascati国家实验室 联合培养博士

工作经历

2020年9月-至今 广东工业大学材料与能源学院 教授

2017年7月-2020年8月 苏州大学 副教授

2016年5月-2017年6月 苏州大学 博士后

2015年3月-2017年4月 美国劳伦斯伯克利国家实验室 博士后

2014年3月-2017年2月 苏州大学 博士后

2013年9月-2014年2月 中科院上海高等研究院 助理研究员

学术兼职

eScience青年编委

主要论文

[1] Y. Feng, Y. Ji, Y. Zhang, Q. Shao,Y. Xu,*Y. Li, X. Huang*. Synthesis of noble metal chalcogenides via cation exchange reactions.Nature Synthesis, 2022, 1, 626–634.

[2] J. Wang, H. Yang, F. Li, L. Li, J. Wu, S. Liu, T. Cheng,Y. Xu,*Q. Shao, X. Huang*, Single-site Pt-doped RuO2 hollow nanospheres with interstitial C for high performance acidic overall water splitting,Science Advances, 2022, 8(9), eabl9271-eabl9271.

[3] T. Yang, X. Mao, Y. Zhang, X. Wu, L. Wang*, M. Chu, C. W. Pao, S. Yang,Y. Xu,*X. Huang*, Coordination tailoring of Cu single sites on C₃N₄ realizes selective CO₂hydrogenation at low temperature,Nature Communications, 2021, 12, 6022.

[4] S. Liu, S. Geng L. Li, Y. Zhang G. Ren, B. Huang*, Z. Hu, J. F. Lee, Y. H. Lai, Y. H. Chu,Y. Xu,*Q. Shao, X. Huang*, A top-down strategy for amorphization of hydroxyl compounds for electrocatalytic oxygen evolution,Nature Communications, 2022, 13, 1187.

[5] S. Bai, F. Liu, B. Huang, F. Li, H. Lin, T. Wu, M. Sun, J. Wu*, Q. Shao, Y. Xu,*X. Huang*, High-efficiency direct methane conversion to oxygenates on a cerium dioxide nanowires supported rhodium single-atom catalyst,Nature Communications, 2020, 11, 954.

[6] S. Bai,Y. Xu,*K. Cao, X. Huang*, Selective Ethanol Oxidation Reaction at the Rh–SnO₂Interface,Advanced Materials, 2021, 33(5), 2005767.

[7] Z. Yu, S. Lv, Q. Yao, N. Fang,Y. Xu,*Q. Shao, C. W. Pao, J. F. Lee, G. Li, L. Yang,* X. Huang,* Low-coordinated Pd site within amorphous palladium selenide for active, selective and stable H₂O₂ electrosynthesis.Advanced Materials, 2023, 35(6), 2208101.

[8] J. Zhang, X. Mao, S. Wang, L. Liang, M. Cao, L. Wang*, G. Li,Y. Xu,* X. Huang*, Hydrogen Evolution Hot Paper Superlattice in a Ru Superstructure for Enhancing Hydrogen Evolution.Angewandte Chemie International Edition 2022, 61, e202116867.

[9] Y. Jin, P. Wang, X. Mao, S. Liu, L. Li, L. Wang*, Q. Shao, Y. Xu,* X. Huang*, A top-down strategy to realize surface reconstruction of small- sized platinum-based nanoparticles for selective hydrogenation,Angewandte Chemie International Edition, 2021, 133(32), 17570-17574.

[10] C. Zhan^#,Y. Xu^#, L. Bu*, H. Zhu, Y. Feng, T. Yang, Y. Zhang, Z. Yang, B. Huang*, Q. Shao, X. Huang*, Subnanometer high-entropy alloy nanowires enable remarkable hydrogen oxidation catalysis,Nature Communications, 2021, 12, 6261.

[11] M. Wang^#,Y. Xu^#, C. Peng, S. Chen, Y. Lin, Z. Hu, L. Sun, S. Ding, C. W. Pao, Q. Shao, X. Huang*, Site-specified two-dimensional heterojunction of Pt nanoparticles/metal-organic frameworks for enhanced hydrogen evolution,Journal of the American Chemical Society, 2021, 143(40), 16512-16518.

[12] J. Zhang, G. Ren, D. Li, Q. Kong, Z. Hu,Y. Xu,*S. Wang, L. Wang,* M. Cao, X. Huang,* Interface engineering of snow-like Ru/RuO₂ nanosheets for boosting hydrogen electrocatalysis.Science Bulletin, 2022, 67, 2103-2111.

[13] H. Peng, T. Yang, H. Lin,Y. Xu,*Z. Wang, Q. Zhang, S. Liu, H. Geng, . Gu, C. Wang, X. Fan,* W. Chen, X. Huang*. Ru/In dual-single atoms modulated charge separation for significantly accelerated photocatalytic H₂ evolution in pure water.Advanced Energy Materials, 2022, 12, 2201688.

[14] S. Liu, Y. Zhang, X. Mao, L. Li, Y. Zhang, L. Li, Y. Pan, X. Li, L. Wang, Q. Shao,Y. Xu,*X. Huang*, Ultrathin perovskite derived Ir-based nanosheets for high-performance electrocatalytic water splitting,Energy & Environmental Science, 2022, 15(4), 1672-1681.

[15] M. Wang, L. Liang, X. Liu, Q. Sun, M. Guo*, S. Bai*,Y. Xu*. Selective semi-hydrogenation of alkynes on palladium-selenium nanocrystals.Journal of Catalysis, 2023, 418, 247-255.

[16] M. Chu, Q. Pan, W. Bian, Y. Liu, M. Cao, C. Zhang, H. Lin,Y. Xu,* Strong metal-support interaction between palladium and gallium oxide within monodisperse nanoparticles, Self-supported catalysts for propyne semi-hydrogenation,Journal of Catalysis, 2021, 395, 36-45.

[17] Y. Dong, Q. Sun, C. Zhan, J. Zhang, H. Yang, T. Cheng,Y. Xu,*Z. Hu, C. W. Pao, H. Geng, X. Huang*, Lattice and Surface Engineering of Ruthenium Nanostructures for Enhanced Hydrogen Oxidation Catalysis.Advanced Functional Materials, 2022, https://doi.org/10.1002/adfm.202210328.

[18] P. Li, X. Liu, M. Guo, Y. Pi*, N. Wang, S. Bai*,Y. Xu,*Qi Sun. Stable and ordered body-centered cubic PdCu phase for highly selective hydrogenation.Small Methods, 2022, 2201356 (front inside cover).

[19] K. Wang, S. Liu, J. Zhang*, Z. Hu, Q. Kong,Y. Xu,*X. Huang*. A one-stone-two-birds strategy to functionalized carbon.ACS Nano, 2022, 16, 15008–15015.

[20] M. Wang, L. Lü, Q. Jiang, G. Li, Q. Hong, M. Wang,Y. Xu,*X. Huang*, Kinetics-Induced Orientational Morphological Evolution of Pd-Sb Rhombohedra from Regular Nanocrystals to Distorted Ones,Science China Materials, 2022,https://doi.org/10.1007/s40843-022-2334-4.

[21] J. Zhang, X. Fan, S. Wang, M. Cao, L. Bu,Y. Xu,*H. Lin*, X. Huang*. Surface engineered Ru₂Ni multilayer nanosheets for hydrogen oxidation catalysis.CCS Chemistry, 2022, 10.31635/ccschem.022.202202269.

[22] L. Ling, M. Chu, R. Song, S. Liu, G. Ren,Y. Xu,*L. Wang*, Q. Xu, Q. Shao, J. Lu*, X. Huang*, CO spillover on ultrathin bimetallic Rh/Rh-M nanosheets.Chem Catalysis, 2022, 2(7),1709-1719.

[23] T. Yang, H. Zhang, C. Zhan, L. Liang,Y. Xu,*P. Ruan, Y. Zhang, J. Li, L. Wang*, X. Lv, S. Yang, C. Pao, X. Huang*. Strong synergy between single atoms and single-atom alloys enables active and selective H₂O₂ synthesis.Chem Catalysis, 2022, 2(12), 3607-3620.

[24] S. Feng, S. Ning, L. Wang, J. Zhao, J. Ou, Z. Wu, S. Luo*, Z. Lin, K. Yan, C. Wu, andY. Xu,*Modifying CsPbX₃(X = Cl, Br, I) with a Zeolitic Imidazolate Framework through Mechanical Milling for Aqueous Photocatalytic H₂Evolution,ACS Appl. Energy Mater.2022, 5, 6248–6255.

[25] Y. Xu*, X. Wang, D. Yang, Z. Tang, M. Cao, H. Hu, L. Wu, L. Liu, J. McLeod, H. Lin*, Y. Li, Y. Lifshitz*, T. K. Sham, Q. Zhang*, Stabilizing oxygen vacancies in ZrO₂by Ga₂O₃boosts the direct dehydrogenation of light alkanes,ACS Catalysis, 2021, 11(16), 10159-10169.

[26] K. Wang, H. Yang, J. Zhang, G. Ren, T. Cheng, Y. Xu,* X. Huang*. The exclusive surface and electronic effects of Ni on promoting the activity of Pt towards alkaline hydrogen oxidation,Nano Research, 2022, 15, 5865–5872.

[27] Q. Yao, Z. Yu, Y. Lai, Y. Chu, T. Chan,Y. Xu,*Q. Shao, X. Huang*, S incorporated RuO₂-based nanorings for active and stable water oxidation in acid,Nano Research, 2022, 15(5), 3964-3970.

[28] Y. Xu,*M. Cao, S. Huang*,Recent advances and perspective on the synthesis and photocatalytic application of metal halide perovskite nanocrystals,Nano Research, 2021, 14(11), 3773-3794.

[29] J. Gong, M. Chu, W. Guan, Y. Liu, Q. Zhong, M. Cao,Y. Xu,*Regulating the interfacial synergy of Ni/Ga₂O₃for CO₂ hydrogenation toward the reverse water–gas shift reaction,Industrial & Engineering Chemistry Research, 2021, 60(26), 9448-9455.

[30] M. Chu, Y. Liu, J. Gong, C. Zhang, X. Wang, Q. Zhong, Li. Wu,Y. Xu,* Suppressing Dehydroisomerization boosts n-butane dehydrogenation with high butadiene Selectivity,Chemistry–A European Journal, 2021, 27(45), 11643-11648.

[31] Q. Yao, B. Huang,Y. Xu,*L. Li, Q. Shao, X. Huang*, A chemical etching strategy to improve and stabilize RuO2-based nanoassemblies for acidic oxygen evolution,Nano Energy, 2021, 84, 105909.

[32] K. Cao, H. Yang, S. Bai,Y. Xu,*C. Yang, Y. Wu, M. Xie, T. Cheng, Q. Shao, X. Huang*, Efficient Direct H₂O₂Synthesis Enabled by PdPb Nanorings via Inhibiting the O−O Bond Cleavage in O₂and H₂O₂, ACS Catalysis, 2021, 11(3), 1106-1118.

[33] L.g Wu, M. Chu, J. Gong, M. Cao*, Y. Liu,Y. Xu,*Regulation of surface carbides on palladium nanocubes with zeolitic imidazolate frameworks for propyne selective hydrogenation,Nano Research, 2021, 14(5), 1559-1564.

[34] W. Ji, C. Zhan,Y. Xu,*D. Li, Y. Zhang, L. Wang , L. Liu , Y. Wang, W. Chen, H. Geng*, X. Huang *, Phase and interface engineering of nickel carbide nanobranches for efficient hydrogen oxidation catalysis,Journal of Materials Chemistry A, 2021, 9(46), 26323-26329.

[35] Y. Pi^#,Y. Xu^#, L. Li, T. Sun, B. Huang, L. Bu, Y. Ma, Z. Hu, C.W. Pao, X. Huang*, Selective surface reconstruction of a defective iridium‐based catalyst for high-efficiency water splitting, Advanced Functional Materials, 2020, 30(43), 2004375 (equal contribution).

[36] Y. Xu,M. Cao, Q. Zhang*, Recent advances and perspective on heterogeneous catalysis using metals and oxide nanocrystals,Materials Chemistry Frontiers, 2021, 5(1), 151-222.

[37] Y. Xu, M. Chu, F. Liu, X. Wang, Y. Liu, M. Cao, J. Gong, J. Luo, H. Lin*, Y. Li, Q. Zhang*, Revealing the correlation between catalytic selectivity and the local coordination environment of Pt single atom,Nano Letters, 2020, 20(9), 6865-6872.

[38] S. Bai, M. Xie, T. Cheng, K. Cao,Y. Xu*, X. Huang*, Surface engineering of RhOOH nanosheets promotes hydrogen evolution in alkaline,Nano Energy, 2020, 78, 105224.

[39] M. Cao, Y. Damji, C. Zhang, L. Wu, Q. Zhong, P. Li, D. Yang, Y. Xu*, Q. Zhang*, Low-Dimensional‐Networked Cesium Lead Halide Perovskites, Properties, Fabrication, and Applications,Small Methods, 2020, 4(12), 2000303.

[40] S. Bai, Q. Yao,Y. Xu*, K. Cao, X. Huang*, Strong synergy in a lichen-like RuCu nanosheet boosts the direct methane oxidation to methanol, Nano Energy, 2020, 71, 104566.

知识产权

[1] 一种丁烷催化脱氢制备丁烯和丁二烯的方法，CN109608301B

[2] 一种低碳烷烃脱氢催化剂及制备低碳烯烃的方法CN109603898B

科研项目

[1] 广东省自然基金杰出青年基金

[2] 国家自然科学基金青年项目

[3] 江苏省自然科学基金青年项目

[4] 江苏省双创博士