徐勇

作者: 时间:2021-03-09 点击数:

 

 

徐勇       教授

所属学院:

材料与能源学院

导师类别:

博士生导师/硕士生导师

科研方向:

纳米催化、能源材料

联系方式:

yongxu@gdut.edu.cn

招生学院:

材料与能源学院

个人简述

课题组聚焦于贵金属纳米催化剂的设计、可控合成、结构调控及构效关系研究。利用多种原位表征方法研究催化剂界面构效关系及催化作用机理,并积极探索在石油化工、新型清洁能源及环境保护等领域的应用。主要研究方向:

1、贵金属纳米催化剂可控合成与结构调控;

2、无机功能纳米催化剂的表界面改性及其在能源与催化方面的应用

学科领域

科学学位:材料科学与工程

专业学位:材料工程

教育背景

20136  中国科学技术大学可再生洁净能源专业  获博士学位

20119-20129月 意大利国家核物理研究院Frascati国家实验室  联合培养博士

工作经历

20209-至今  广东工业大学材料与能源学院  教授

20177-20208  苏州大学  副教授

20165-20176  苏州大学  博士后

20153-20174  美国劳伦斯伯克利国家实验室  博士后

20143-20172  苏州大学  博士后

20139-20142  中科院上海高等研究院  助理研究员

学术兼职

eScience青年编委

 

 

主要论文

[1]   Y. Feng, Y. Ji, Y. Zhang, Q. Shao, Y. Xu,* Y. Li, X. Huang*. Synthesis   of noble metal chalcogenides via cation exchange reactions. Nature Synthesis, 2022, 1, 626–634.

[2]   J. Wang, H. Yang, F. Li, L. Li, J. Wu, S. Liu, T. Cheng, Y. Xu,* Q.   Shao, X. Huang*, Single-site Pt-doped RuO2 hollow nanospheres with   interstitial C for high performance acidic overall water splitting, Science Advances, 2022, 8(9), eabl9271-eabl9271.

[3]   T. Yang, X. Mao, Y. Zhang, X. Wu, L. Wang*, M. Chu, C. W. Pao, S. Yang, Y.   Xu,* X. Huang*, Coordination tailoring of Cu single sites on C3N4   realizes selective CO2 hydrogenation at low temperature, Nature Communications, 2021, 12, 6022.

[4]   S. Liu, S. Geng L. Li, Y. Zhang G. Ren, B. Huang*, Z. Hu, J. F. Lee, Y. H.   Lai, Y. H. Chu, Y. Xu,* Q. Shao, X. Huang*, A top-down strategy for   amorphization of hydroxyl compounds for electrocatalytic oxygen evolution, Nature Communications, 2022, 13, 1187.

[5]   S. Bai, F. Liu, B. Huang, F. Li, H. Lin, T. Wu, M. Sun, J. Wu*, Q. Shao,   Y. Xu,* X. Huang*, High-efficiency direct methane conversion to   oxygenates on a cerium dioxide nanowires supported rhodium single-atom   catalyst, Nature Communications, 2020,   11, 954.

[6]   S. Bai, Y. Xu,* K. Cao, X. Huang*, Selective Ethanol Oxidation   Reaction at the Rh–SnO2 Interface, Advanced   Materials, 2021, 33(5), 2005767.

[7]   Z. Yu, S. Lv, Q. Yao, N. Fang, Y. Xu,* Q. Shao, C. W. Pao, J. F. Lee,   G. Li, L. Yang,* X. Huang,* Low-coordinated Pd site within amorphous   palladium selenide for active, selective and stable H2O2   electrosynthesis. Advanced Materials,   2023, 35(6), 2208101.

[8]   J. Zhang, X. Mao, S. Wang, L. Liang, M. Cao, L. Wang*, G. Li, Y. Xu,*   X. Huang*, Hydrogen Evolution Hot Paper Superlattice in a Ru Superstructure   for Enhancing Hydrogen Evolution. Angewandte   Chemie International Edition 2022, 61, e202116867.

[9]   Y. Jin, P. Wang, X. Mao, S. Liu, L. Li, L. Wang*, Q. Shao, Y. Xu,* X. Huang*,   A top-down strategy to realize surface reconstruction of small- sized   platinum-based nanoparticles for selective hydrogenation, Angewandte Chemie International Edition, 2021,   133(32), 17570-17574.

[10]   C. Zhan#, Y. Xu#, L. Bu*, H. Zhu, Y. Feng, T.   Yang, Y. Zhang, Z. Yang, B. Huang*, Q. Shao, X. Huang*, Subnanometer   high-entropy alloy nanowires enable remarkable hydrogen oxidation catalysis, Nature Communications, 2021, 12, 6261.

[11]   M. Wang#, Y. Xu#, C. Peng, S. Chen, Y. Lin, Z.   Hu, L. Sun, S. Ding, C. W. Pao, Q. Shao, X. Huang*, Site-specified   two-dimensional heterojunction of Pt nanoparticles/metal-organic frameworks   for enhanced hydrogen evolution, Journal of the   American Chemical Society, 2021, 143(40), 16512-16518.

[12]   J. Zhang, G. Ren, D. Li, Q. Kong, Z. Hu, Y. Xu,* S. Wang, L. Wang,* M.   Cao, X. Huang,* Interface engineering of snow-like Ru/RuO2   nanosheets for boosting hydrogen electrocatalysis. Science Bulletin, 2022, 67, 2103-2111.

[13]   H. Peng, T. Yang, H. Lin, Y. Xu,* Z. Wang, Q. Zhang, S. Liu, H. Geng,   . Gu, C. Wang, X. Fan,* W. Chen, X. Huang*. Ru/In dual-single atoms modulated   charge separation for significantly accelerated photocatalytic H2   evolution in pure water. Advanced Energy Materials,   2022, 12, 2201688.

[14]   S. Liu, Y. Zhang, X. Mao, L. Li, Y. Zhang, L. Li, Y. Pan, X. Li, L. Wang, Q.   Shao, Y. Xu,* X. Huang*, Ultrathin perovskite derived Ir-based   nanosheets for high-performance electrocatalytic water splitting, Energy & Environmental Science, 2022, 15(4),   1672-1681.

[15]   M. Wang, L. Liang, X. Liu, Q. Sun, M. Guo*, S. Bai*, Y. Xu*. Selective   semi-hydrogenation of alkynes on palladium-selenium nanocrystals. Journal   of Catalysis, 2023, 418, 247-255.

[16]   M. Chu, Q. Pan, W. Bian, Y. Liu, M. Cao, C. Zhang, H. Lin, Y. Xu,*   Strong metal-support interaction between palladium and gallium oxide within   monodisperse nanoparticles, Self-supported catalysts for propyne   semi-hydrogenation, Journal of Catalysis, 2021, 395, 36-45.

[17]   Y. Dong, Q. Sun, C. Zhan, J. Zhang, H. Yang, T. Cheng, Y. Xu,* Z. Hu,   C. W. Pao, H. Geng, X. Huang*, Lattice and Surface Engineering of Ruthenium   Nanostructures for Enhanced Hydrogen Oxidation Catalysis. Advanced   Functional Materials, 2022, https://doi.org/10.1002/adfm.202210328.

[18]   P. Li, X. Liu, M. Guo, Y. Pi*, N. Wang, S. Bai*, Y. Xu,* Qi Sun.   Stable and ordered body-centered cubic PdCu phase for highly selective   hydrogenation. Small Methods, 2022,   2201356 (front inside cover).

[19]   K. Wang, S. Liu, J. Zhang*, Z. Hu, Q. Kong, Y. Xu,* X. Huang*. A   one-stone-two-birds strategy to functionalized carbon. ACS Nano, 2022, 16, 15008–15015.

[20]   M. Wang, L. Lü, Q. Jiang, G. Li, Q. Hong, M. Wang, Y. Xu,* X. Huang*,   Kinetics-Induced Orientational Morphological Evolution of Pd-Sb Rhombohedra   from Regular Nanocrystals to Distorted Ones, Science   China Materials, 2022, https://doi.org/10.1007/s40843-022-2334-4.

[21]   J. Zhang, X. Fan, S. Wang, M. Cao, L. Bu, Y. Xu,* H. Lin*, X. Huang*.   Surface engineered Ru2Ni multilayer nanosheets for hydrogen   oxidation catalysis. CCS Chemistry,   2022, 10.31635/ccschem.022.202202269.

[22]   L. Ling, M. Chu, R. Song, S. Liu, G. Ren, Y. Xu,* L. Wang*, Q. Xu, Q.   Shao, J. Lu*, X. Huang*, CO spillover on ultrathin bimetallic Rh/Rh-M   nanosheets. Chem Catalysis, 2022,   2(7),1709-1719.

[23]   T. Yang, H. Zhang, C. Zhan, L. Liang, Y. Xu,* P. Ruan, Y. Zhang, J.   Li, L. Wang*, X. Lv, S. Yang, C. Pao, X. Huang*. Strong synergy between   single atoms and single-atom alloys enables active and selective H2O2   synthesis. Chem Catalysis, 2022,   2(12), 3607-3620.

[24]   S. Feng, S. Ning, L. Wang, J. Zhao, J. Ou, Z. Wu, S. Luo*, Z. Lin, K. Yan, C.   Wu, and Y. Xu,* Modifying CsPbX3 (X = Cl, Br, I) with a   Zeolitic Imidazolate Framework through Mechanical Milling for Aqueous   Photocatalytic H2 Evolution, ACS Appl. Energy Mater. 2022,   5, 6248–6255.

[25]   Y. Xu*, X. Wang, D. Yang, Z. Tang, M. Cao, H. Hu, L. Wu, L. Liu, J.   McLeod, H. Lin*, Y. Li, Y. Lifshitz*, T. K. Sham, Q. Zhang*, Stabilizing   oxygen vacancies in ZrO2 by Ga2O3 boosts the   direct dehydrogenation of light alkanes, ACS Catalysis, 2021, 11(16),   10159-10169.

[26]   K. Wang, H. Yang, J. Zhang, G. Ren, T. Cheng, Y. Xu,* X. Huang*. The   exclusive surface and electronic effects of Ni on promoting the activity of   Pt towards alkaline hydrogen oxidation, Nano Research, 2022, 15,   5865–5872.

[27]   Q. Yao, Z. Yu, Y. Lai, Y. Chu, T. Chan, Y. Xu,* Q. Shao, X. Huang*, S   incorporated RuO2-based nanorings for active and stable water   oxidation in acid, Nano Research, 2022, 15(5), 3964-3970.

[28]   Y. Xu,* M. Cao, S. Huang*,Recent advances and perspective on the   synthesis and photocatalytic application of metal halide perovskite   nanocrystals, Nano Research, 2021, 14(11), 3773-3794.

[29]   J. Gong, M. Chu, W. Guan, Y. Liu, Q. Zhong, M. Cao, Y. Xu,* Regulating   the interfacial synergy of Ni/Ga2O3 for CO2   hydrogenation toward the reverse water–gas shift reaction, Industrial   & Engineering Chemistry Research, 2021, 60(26), 9448-9455.

[30]   M. Chu, Y. Liu, J. Gong, C. Zhang, X. Wang, Q. Zhong, Li. Wu, Y. Xu,*   Suppressing Dehydroisomerization boosts n-butane dehydrogenation with high   butadiene Selectivity, Chemistry–A European Journal, 2021, 27(45),   11643-11648.

[31]   Q. Yao, B. Huang, Y. Xu,* L. Li, Q. Shao, X. Huang*, A chemical   etching strategy to improve and stabilize RuO2-based nanoassemblies for   acidic oxygen evolution, Nano Energy, 2021, 84, 105909.

[32]   K. Cao, H. Yang, S. Bai, Y. Xu,* C. Yang, Y. Wu, M. Xie, T. Cheng, Q.   Shao, X. Huang*, Efficient Direct H2O2 Synthesis   Enabled by PdPb Nanorings via Inhibiting the OO Bond Cleavage in O2 and H2O2,   ACS Catalysis, 2021, 11(3), 1106-1118.

[33]   L.g Wu, M. Chu, J. Gong, M. Cao*, Y. Liu, Y. Xu,* Regulation of   surface carbides on palladium nanocubes with zeolitic imidazolate frameworks   for propyne selective hydrogenation, Nano Research, 2021, 14(5),   1559-1564.

[34]   W. Ji, C. Zhan, Y. Xu,* D. Li, Y. Zhang, L. Wang , L. Liu , Y. Wang, W.   Chen, H. Geng*, X. Huang *, Phase and interface engineering of nickel carbide   nanobranches for efficient hydrogen oxidation catalysis, Journal of   Materials Chemistry A, 2021, 9(46), 26323-26329.

[35]   Y. Pi#, Y. Xu#, L. Li, T. Sun, B. Huang, L. Bu,   Y. Ma, Z. Hu, C.W. Pao, X. Huang*, Selective surface reconstruction of a   defective iridium‐based catalyst for high-efficiency water splitting,   Advanced Functional Materials, 2020, 30(43), 2004375 (equal   contribution).

[36]   Y. Xu, M. Cao, Q. Zhang*, Recent advances and perspective on   heterogeneous catalysis using metals and oxide nanocrystals, Materials   Chemistry Frontiers, 2021, 5(1), 151-222.

[37]   Y. Xu, M. Chu, F. Liu, X. Wang, Y. Liu, M. Cao, J. Gong, J. Luo, H.   Lin*, Y. Li, Q. Zhang*, Revealing the correlation between catalytic   selectivity and the local coordination environment of Pt single atom, Nano   Letters, 2020, 20(9), 6865-6872.

[38]   S. Bai, M. Xie, T. Cheng, K. Cao, Y. Xu*, X. Huang*, Surface   engineering of RhOOH nanosheets promotes hydrogen evolution in alkaline, Nano   Energy, 2020, 78, 105224.

[39]   M. Cao, Y. Damji, C. Zhang, L. Wu, Q. Zhong, P. Li, D. Yang, Y. Xu*, Q.   Zhang*, Low-Dimensional‐Networked Cesium Lead Halide Perovskites, Properties,   Fabrication, and Applications, Small Methods, 2020, 4(12), 2000303.

 

[40]   S. Bai, Q. Yao, Y. Xu*, K. Cao, X. Huang*, Strong synergy in a   lichen-like RuCu nanosheet boosts the direct methane oxidation to methanol,   Nano Energy, 2020, 71, 104566.

 

知识产权

[1]   一种丁烷催化脱氢制备丁烯和丁二烯的方法,CN109608301B

[2]   一种低碳烷烃脱氢催化剂及制备低碳烯烃的方法 CN109603898B

 

科研项目

[1]   广东省自然基金杰出青年基金

[2]   国家自然科学基金青年项目

[3]   江苏省自然科学基金青年项目

[4]   江苏省双创博士

 





 

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